diff --git a/docs/source/llm/export-llm-optimum.md b/docs/source/llm/export-llm-optimum.md
new file mode 100644
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+# Exporting LLMs with HuggingFace's Optimum ExecuTorch
+
+[Optimum ExecuTorch](https://github.com/huggingface/optimum-executorch) provides a streamlined way to export Hugging Face transformer models to ExecuTorch format. It offers seamless integration with the Hugging Face ecosystem, making it easy to export models directly from the Hugging Face Hub.
+
+## Overview
+
+Optimum ExecuTorch supports a much wider variety of model architectures compared to ExecuTorch's native `export_llm` API. While `export_llm` focuses on a limited set of highly optimized models (Llama, Qwen, Phi, and SmolLM) with advanced features like SpinQuant and attention sink, Optimum ExecuTorch can export diverse architectures including Gemma, Mistral, GPT-2, BERT, T5, Whisper, Voxtral, and many others.
+
+### Use Optimum ExecuTorch when:
+- You need to export models beyond the limited set supported by `export_llm`
+- Exporting directly from Hugging Face Hub model IDs, including model variants such as finetunes
+- You want a simpler interface with Hugging Face ecosystem integration
+
+### Use export_llm when:
+- Working with one of the highly optimized supported models (Llama, Qwen, Phi, SmolLM)
+- You need advanced optimizations like SpinQuant or attention sink
+- You need pt2e quantization for QNN/CoreML/Vulkan backends
+- Working with Llama models requiring custom checkpoints
+
+See [Exporting LLMs](export-llm.md) for details on using the native `export_llm` API.
+
+## Prerequisites
+
+### Installation
+
+First, clone and install Optimum ExecuTorch from source:
+
+```bash
+git clone https://github.com/huggingface/optimum-executorch.git
+cd optimum-executorch
+pip install '.[dev]'
+```
+
+For access to the latest features and optimizations, install dependencies in dev mode:
+
+```bash
+python install_dev.py
+```
+
+This installs `executorch`, `torch`, `torchao`, `transformers`, and other dependencies from nightly builds or source.
+
+## Supported Models
+
+Optimum ExecuTorch supports a wide range of model architectures including decoder-only LLMs (Llama, Qwen, Gemma, Mistral, etc.), multimodal models, vision models, audio models (Whisper), encoder models (BERT, RoBERTa), and seq2seq models (T5).
+
+For the complete list of supported models, see the [Optimum ExecuTorch documentation](https://github.com/huggingface/optimum-executorch#-supported-models).
+
+## Export Methods
+
+Optimum ExecuTorch offers two ways to export models:
+
+### Method 1: CLI Export
+
+The CLI is the simplest way to export models. It provides a single command to convert models from Hugging Face Hub to ExecuTorch format.
+
+#### Basic Export
+
+```bash
+optimum-cli export executorch \
+    --model "HuggingFaceTB/SmolLM2-135M-Instruct" \
+    --task "text-generation" \
+    --recipe "xnnpack" \
+    --output_dir="./smollm2_exported"
+```
+
+#### With Optimizations
+
+Add custom SDPA, KV cache optimization, and quantization:
+
+```bash
+optimum-cli export executorch \
+    --model "HuggingFaceTB/SmolLM2-135M-Instruct" \
+    --task "text-generation" \
+    --recipe "xnnpack" \
+    --use_custom_sdpa \
+    --use_custom_kv_cache \
+    --qlinear 8da4w \
+    --qembedding 8w \
+    --output_dir="./smollm2_exported"
+```
+
+#### Available CLI Arguments
+
+Key arguments for LLM export include `--model`, `--task`, `--recipe` (backend), `--use_custom_sdpa`, `--use_custom_kv_cache`, `--qlinear` (linear quantization), `--qembedding` (embedding quantization), and `--max_seq_len`.
+
+For the complete list of arguments, run:
+```bash
+optimum-cli export executorch --help
+```
+
+## Optimization Options
+
+### Custom Operators
+
+Optimum ExecuTorch includes custom SDPA (~3x speedup) and custom KV cache (~2.5x speedup) operators. Enable with `--use_custom_sdpa` and `--use_custom_kv_cache`.
+
+### Quantization
+
+Optimum ExecuTorch uses [TorchAO](https://github.com/pytorch/ao) for quantization. Common options:
+- `--qlinear 8da4w`: int8 dynamic activation + int4 weight (recommended)
+- `--qembedding 4w` or `--qembedding 8w`: int4/int8 embedding quantization
+
+Example:
+```bash
+optimum-cli export executorch \
+    --model "meta-llama/Llama-3.2-1B" \
+    --task "text-generation" \
+    --recipe "xnnpack" \
+    --use_custom_sdpa \
+    --use_custom_kv_cache \
+    --qlinear 8da4w \
+    --qembedding 4w \
+    --output_dir="./llama32_1b"
+```
+
+### Backend Support
+
+Supported backends: `xnnpack` (CPU), `coreml` (Apple GPU), `portable` (baseline), `cuda` (NVIDIA GPU). Specify with `--recipe`.
+
+## Exporting Different Model Types
+
+Optimum ExecuTorch supports various model architectures with different tasks:
+
+- **Decoder-only LLMs**: Use `--task text-generation`
+- **Multimodal LLMs**: Use `--task multimodal-text-to-text`
+- **Seq2Seq models** (T5): Use `--task text2text-generation`
+- **ASR models** (Whisper): Use `--task automatic-speech-recognition`
+
+For detailed examples of exporting each model type, see the [Optimum ExecuTorch export guide](https://github.com/huggingface/optimum-executorch/blob/main/optimum/exporters/executorch/README.md).
+
+## Running Exported Models
+
+### Verifying Output with Python
+
+After exporting, you can verify the model output in Python before deploying to device using classes from `modeling.py`, such as the `ExecuTorchModelForCausalLM` class for LLMs:
+
+```python
+from optimum.executorch import ExecuTorchModelForCausalLM
+from transformers import AutoTokenizer
+
+# Load the exported model
+model = ExecuTorchModelForCausalLM.from_pretrained("./smollm2_exported")
+tokenizer = AutoTokenizer.from_pretrained("HuggingFaceTB/SmolLM2-135M-Instruct")
+
+# Generate text
+generated_text = model.text_generation(
+    tokenizer=tokenizer,
+    prompt="Once upon a time",
+    max_seq_len=128,
+)
+print(generated_text)
+```
+
+### Running on Device
+
+After verifying your model works correctly, deploy it to device:
+
+- [Running with C++](run-with-c-plus-plus.md) - Run exported models using ExecuTorch's C++ runtime
+- [Running on Android](https://github.com/meta-pytorch/executorch-examples/tree/main/llm/android) - Deploy to Android devices
+- [Running on iOS](https://github.com/meta-pytorch/executorch-examples/tree/main/llm/apple) - Deploy to iOS devices
+
+## Performance
+
+For performance benchmarks and on-device metrics, see the [Optimum ExecuTorch benchmarks](https://github.com/huggingface/optimum-executorch#-benchmarks-on-mobile-devices) and the [ExecuTorch Benchmark Dashboard](https://hud.pytorch.org/benchmark/llms?repoName=pytorch%2Fexecutorch).
+
+## Additional Resources
+
+- [Optimum ExecuTorch GitHub](https://github.com/huggingface/optimum-executorch) - Full documentation and examples
+- [Supported Models](https://github.com/huggingface/optimum-executorch#-supported-models) - Complete model list
+- [Export Guide](https://github.com/huggingface/optimum-executorch/blob/main/optimum/exporters/executorch/README.md) - Detailed export examples
+- [TorchAO Quantization](https://github.com/pytorch/ao) - Quantization library documentation
diff --git a/docs/source/llm/export-llm.md b/docs/source/llm/export-llm.md
index e9f8307f2c3..c5d0631b547 100644
--- a/docs/source/llm/export-llm.md
+++ b/docs/source/llm/export-llm.md
@@ -20,6 +20,8 @@ As of this doc, the list of supported LLMs include the following:
 
 The up-to-date list of supported LLMs can be found in the code [here](https://github.com/pytorch/executorch/blob/main/extension/llm/export/config/llm_config.py#L32).
 
+**Note:** If you need to export models that are not on this list or other model architectures (such as Gemma, Mistral, BERT, T5, Whisper, etc.), see [Exporting LLMs with Optimum](export-llm-optimum.md) which supports a much wider variety of models from Hugging Face Hub.
+
 ## The export_llm API
 `export_llm` is ExecuTorch's high-level export API for LLMs. In this tutorial, we will focus on exporting Llama 3.2 1B using this API. `export_llm`'s arguments are specified either through CLI args or through a yaml configuration whose fields are defined in [`LlmConfig`](https://github.com/pytorch/executorch/blob/main/extension/llm/export/config/llm_config.py). To call `export_llm`:
 
diff --git a/docs/source/llm/getting-started.md b/docs/source/llm/getting-started.md
index 6b6f9d96df7..95caae6ddd9 100644
--- a/docs/source/llm/getting-started.md
+++ b/docs/source/llm/getting-started.md
@@ -18,8 +18,12 @@ To follow this guide, you'll need to install ExecuTorch. Please see [Setting Up
 
 Deploying LLMs to ExecuTorch can be boiled down to a two-step process: (1) exporting the LLM to a `.pte` file and (2) running the `.pte` file using our C++ APIs or Swift/Java bindings.
 
-- [Exporting LLMs](export-llm.md)
+### Exporting
+- [Exporting LLMs](export-llm.md) - Export using ExecuTorch's native `export_llm` API with advanced optimizations
+- [Exporting LLMs with Optimum](export-llm-optimum.md) - Export Hugging Face models with broader architecture support
 - [Exporting custom LLMs](export-custom-llm.md)
+
+### Running
 - [Running with C++](run-with-c-plus-plus.md)
 - [Running on Android (XNNPack)](https://github.com/meta-pytorch/executorch-examples/tree/main/llm/android)
 - [Running on Android (Qualcomm)](build-run-llama3-qualcomm-ai-engine-direct-backend.md)
diff --git a/docs/source/llm/working-with-llms.md b/docs/source/llm/working-with-llms.md
index 4c238f7ae5c..e4088efd12b 100644
--- a/docs/source/llm/working-with-llms.md
+++ b/docs/source/llm/working-with-llms.md
@@ -11,6 +11,7 @@ Learn how to export LLM models and deploy them across different platforms and ru
 
 getting-started
 export-llm
+export-llm-optimum
 export-custom-llm
 run-with-c-plus-plus
 build-run-llama3-qualcomm-ai-engine-direct-backend